FasV

Enzyme Information
reference: 10.1002/anie.202418843
host: E. coli (DE3)
phmm-model: FDH_conventional.hmm
halide-source: NaCl

Gene Data
phmm effect mutation gene_name reference
- weak halogenation activity L309E FasV DOI: 10.1002/anie.202418843
- exclusively catalyses selective monohalogenation I212T FasV DOI: 10.1002/anie.202418843
- significant decrease in halogenation activity S310A FasV DOI: 10.1002/anie.202418843
- significant decrease in halogenation activity S310D FasV DOI: 10.1002/anie.202418843
- significant decrease in halogenation activity S310T FasV DOI: 10.1002/anie.202418843
29 directly acts as a base to activate the hydroxy group at the ortho position of the halogenation site; dual activation mechanism E49 FasV DOI: 10.1002/anie.202418843
- reduction in halogenation activity E49A FasV DOI: 10.1002/anie.202418843
- reduction in halogenation activity E49D FasV DOI: 10.1002/anie.202418843
- reduction in halogenation activity E49Q FasV DOI: 10.1002/anie.202418843
- complete loss of activity S50A FasV DOI: 10.1002/anie.202418843
- complete loss of activity S50V FasV DOI: 10.1002/anie.202418843
- complete loss of activity S50E FasV DOI: 10.1002/anie.202418843
- accumulation of dichlorinated compound (11) F93W FasV DOI: 10.1002/anie.202418843
- lost polychlorination activity L81A FasV DOI: 10.1002/anie.202418843
- similar regioselectivity with compound 1 and 3 L81Y FasV DOI: 10.1002/anie.202418843
- when incubated with 1 or 3, there was a higher production of intermediate 5 and abolishment of 11; stricter regioselectivity and reduces the diversion toward other halogenation routes T53A FasV DOI: 10.1002/anie.202418843
- accumulated more compound 2 and a monochlorinated compound I212L FasV DOI: 10.1002/anie.202418843
- no polychlorination activity I212T FasV DOI: 10.1002/anie.202418843
295 H-network around substrate; likely hydrophobic pocket formation L309 FasV DOI: 10.1002/anie.202418843
198 H-network around substrate; binding of monochlorinated compound and subsequent polychlorination I212 FasV DOI: 10.1002/anie.202418843
- conserved in homologous proteins; 212 is partially conserved featuring predominantly Ile and Thr residues G209-D231 FasV DOI: 10.1002/anie.202418843
134 substrate binding; dual activation mechanism S150 FasV DOI: 10.1002/anie.202418843
77 H-network around substrate; crucial for substrate binding F93 FasV DOI: 10.1002/anie.202418843
33 crucial for substrate binding T53 FasV DOI: 10.1002/anie.202418843
30 might promote the electrophilic addition of chloride to the substrate; catalytic activity S50 FasV DOI: 10.1002/anie.202418843
77 might be responsible for regioselectivity by regulating substrate binding F93 FasV DOI: 10.1002/anie.202418843
57 catalytic activity; dual activation mechanism K76 FasV DOI: 10.1002/anie.202418843
- weak halogenation activity L309A FasV DOI: 10.1002/anie.202418843